Thioether-ligated iron(II) and iron(III)-hydroperoxo/alkylperoxo complexes with an H-bond donor in the second coordination sphere.

نویسندگان

  • Leland R Widger
  • Yunbo Jiang
  • Alison C McQuilken
  • Tzuhsiung Yang
  • Maxime A Siegler
  • Hirotoshi Matsumura
  • Pierre Moënne-Loccoz
  • Devesh Kumar
  • Sam P de Visser
  • David P Goldberg
چکیده

The non-heme iron complexes, [Fe(II)(N3PySR)(CH3CN)](BF4)2 () and [Fe(II)(N3Py(amide)SR)](BF4)2 (), afford rare examples of metastable Fe(iii)-OOH and Fe(iii)-OOtBu complexes containing equatorial thioether ligands and a single H-bond donor in the second coordination sphere. These peroxo complexes were characterized by a range of spectroscopic methods and density functional theory studies. The influence of a thioether ligand and of one H-bond donor on the stability and spectroscopic properties of these complexes was investigated.

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عنوان ژورنال:
  • Dalton transactions

دوره 43 20  شماره 

صفحات  -

تاریخ انتشار 2014